vestichИзвестия Национальной академии наук Беларуси. Серия химических наукProceedings of the National Academy of Sciences of Belarus, Chemical Series1561-83312524-2342The Republican Unitary Enterprise Publishing House "Belaruskaya Navuka"vestich-295Research ArticleОБЗОРЫГЕТЕРОЦИКЛИЧЕСКИЕ ПРОИЗВОДНЫЕ МЕТАЛЛОЦЕНОВHETEROCYCLES DERIVATIVES OF METALLOCENESКолесникИ. А.KolesnikI. A.

мл. науч. сотрудник

ул. Сурганова, 13, 220072

Junior Researcher

13, Surganov Str., 220072

zvetok_kaktusa@mail.ruДикусарЕ. А.DikusarE. A.

канд. хим. наук, ст. науч. сотрудник

ул. Сурганова, 13, 220072

Ph. D. (Chemistry), Senior Researcher

13, Surganov Str., 220072

dikusar@ifoch.bas-net.byИнститут физико-органической химии НАН Беларуси, МинскInstitute of Physical Organic Chemistry of the National Academy of Sciences of Belarus, Minsk20171412201704107125Copyright © Колесник И.А., Дикусар Е.А., 20172017Колесник И.А., Дикусар Е.А.Kolesnik I.A., Dikusar E.A.Данная работа распространяется под лицензией Creative Commons Attribution 4.0.This work is licensed under a Creative Commons Attribution 4.0 License.https://vestichem.belnauka.by/jour/article/view/295

Обзор посвящен методологии получения производных металлоценов, содержащих гетероциклические фрагменты, что позволяет не только усилить специфическое действие и свойства последних, но и получать соединения с принципиально новыми свойствами. Изоксазол входит в состав множества природных биологически активных соединений, его производные используются для лечения заболеваний центральной нервной системы, как противоопухолевые агенты, анальгетики, анестетики, миорелаксанты, антибиотики. Целенаправленно синтезированные производные изотиазола проявляют противовирусную, противораковую, антибиотическую активность, являются эффективными иммунодепрессантами, противовоспалительными и противотромбозными средствами. Производные указанных азолов занимают особое место в агрохимии в качестве гербицидов, пестицидов, инсектицидов или фунгицидов. В свою очередь соединения ферроцена представляют интерес ввиду широкого спектра их химических превращений и разнообразных путей практического использования в технике, электрохимии, катализе, а также в биологии и медицине. Более того, отмечено, что включение ферроценового фрагмента в органическую молекулу зачастую приводит к возникновению совершенно новых свойств и в том числе – биологической активности. Это обусловлено увеличением скорости проникновения вещества через клеточные мембраны из-за высокой липофильности ферроценового фрагмента, а следовательно, протеканием аномального метаболизма ферроценсодержащего соединения. Не менее разнообразны и направления применения цимантреновых производных; однако использование биологически активных соединений на его основе ограничено по причине достаточно высокой токсичности цимантренового фрагмента. Большой интерес представляет способность цимантреновой структуры к переметаллированию с образованием производных других металлоценов. 

The review article is devoted to the methodology of getting derivatives containing metallocene and heterocyclic fragments united in one molecule, which allows not only strengthening the specific action and the properties of the latter, but also obtaining compounds with radically new properties. Isoxazole is a part of many biologically active compounds, and its derivatives are used to treat diseases of the central nervous system, such as anti-tumor agents, analgesics, anesthetics, muscle relaxants, antibiotics. Purposefully synthesized isothiazole derivatives exhibit antiviral, anticancer, antibiotic activity, are effective immunosuppressive drugs, anti-inflammatory and antithrombotic agents. Derivatives of these azoles have a special place in agrochemicals as herbicides, pesticides, insecticides or fungicides. In turn, ferrocene compounds are of interest due to their wide range of chemical transformations and various ways of practical use in the art of electrochemistry, catalysis, and also in medicine and biology. Moreover, it is noted that the inclusion of the ferrocene moiety in an organic molecule often leads to completely new properties, including biological activity. This is due to the increase of penetration rate of material through the cell membranes due to the high lipophilicity of the ferrocene moiety, and therefore, the occurrence of abnormal metabolism ferrocene compound. Cymantrene derivatives applications are no less diverse; however, the use of biologically active compounds based on it is limited because of quite high toxicity of cymantrene fragment. Of great interest is the ability of the cymantrene structure to transmetallation with the formation of derivatives of other metallocenes. 

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The authors declare that there are no conflicts of interest present.